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One of the most striking signatures of Weyl fermions in solid-state systems is their surface Fermi arcs. Fermi arcs can also be localized at internal twin boundaries where two Weyl materials of opposite chirality meet. In this work, we derive constraints on the topology and connectivity of these “internal Fermi arcs.” We show that internal Fermi arcs can exhibit transport signatures, and we propose two probes: quantum oscillations and a quantized chiral magnetic current. We propose merohedrally twinned B20 materials as candidates to host internal Fermi arcs, verified through both model and calculations. Our theoretical investigation sheds light on the topological features and motivates experimental studies on the intriguing physics of internal Fermi arcs. 

The solid solution LnSbxTe2−x−δ (Ln = lanthanide) is a family of square-net topological semimetals that exhibit tunable charge density wave (CDW) distortions and band filling dependent on x, offering broad opportunities to examine the interplay of topological electronic states, CDW, and magnetism. While several Ln series have been characterized, gaps in the literature remain, inviting a systematic survey of the remaining composition space that is synthetically accessible. We present our efforts to synthesize LnSbxTe2−x−δ across the remaining lanthanides via chemical vapor transport. Compiling our results with the reported literature, we generate a stability phase diagram across the ranges of Ln and x. We find a stability boundary for intermediate x beyond Tb, while x = 1 and x = 0 can be isolated up to Ho and Dy, respectively. SEM and XRD analyses of unsuccessful reactions indicated the formation of several stable binary phases. The presence of structurally related LnTe3 in samples suggests that stability is limited by the size of Ln, due to increasing compressive strain along the layer stacking axis with decreasing size. Finally, we demonstrate that late Ln can be stabilized in LnSbxTe2−x−δ via substitution into larger Ln members, synthesizing La1−yHoySbxTe2−x−δ as a proof of concept. 

Freestanding monolayer CrOCl nanosheet obtainedviachemical exfoliation for the first time.